DISTRIBUTIONS AND VARIATIONS OF SURFACE OZONE IN CHANGSHU,YANGTZE DELTA REGION

(整期优先)网络出版时间:2003-02-12
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Throughoneandhalfyearcontinuousin-situmeasurements,thedistributionsandvariationsofsurfaceozoneanditsprecursorsatatypicalmixedagriculturalandmetropolitanarea-Changshu,YangtzeDeltaregion,werestudied.Thepreliminaryanalysisontheconcentrationlevelsandvariationsofsurfaceozoneindicatedtheobviousseasonalanddiurnalcyclesduringtheexperiment.Thehourlyaveragedconcentrationsofsurfaceozonewerehigh,inabout17%oftotalvalidhoursthesurfaceozoneconcentrationexceeded50ppb,andin22daysthehourlyaveragedozoneconcentrationwasgreaterthan100ppb.Therewereabout40%ofthedaysinthatthedailymaximum8-hourozoneconcentrationwasgreaterthan50ppb.Thedayswithdailymaximum8-hourozoneconcentrationgreaterthan80ppbwereabout33daysthataccountedforabout8%oftheobservationaldays.Thevariationsof5-daymovingaveragedozoneconcentrationsdependedbothontheweatherconditionsandonthechangesofozoneinbackgroundatmosphere.Photochemicalprocesshadthesignificantimpactsonozoneproductions.