简介：Tuningthecoloroutputofrare-earthiondopedluminescentnanomaterialshasimportantscientificsignificanceforfurtherextendingapplicationsincolordisplays,lasersources,optoelectronicdevices,andbiolabeling.Inpreviousstudies,pre-designedphasemodulationofthefemtosecondlaserfieldhasbeenproventobeeffectiveintuningtheluminescenceofdopedrare-earthions.Owingtothecomplexlight–matterinteractionintheactualexperiment,thedynamicrangeandoptimalefficiencyforcolortuningcannotbedeterminedwiththepre-designedphasemodulation.Thisarticlesharesthedevelopmentofanadaptivefemtosecondpulseshapingmethodbasedonageneticalgorithm,anditsusetomanipulatethegreenandredluminescencetuninginanEr3+-dopedglassceramicunder800-nmfemtosecondlaserfieldexcitationforthefirsttime.ExperimentalresultsshowthattheintensityratioofthegreenandredUCluminescenceofthedopedEr3+ionscanbeeitherincreasedordecreasedconvenientlybythephase-shapedfemtosecondlaserfieldwithanoptimalfeedbackcontrol.Thephysicalcontrolmechanismsforthecolortuningarealsoexplainedindetail.Thisarticledemonstratesthepotentialapplicationsoftheadaptivefemtosecondpulseshapingtechniqueincontrollingthecoloroutputofdopedrare-earthions.