Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of Wuhan-中国期刊网

摘要 TheimpactofBrownCarbon(BrC)toaerosollightabsorptionhasbeenpaidmoreattentionrecentlyandtherearealargenumberofstudiesshowingthattheinfluenceofBrConradiativeforcingshouldnotbeignored.BrCalsoactsasanimportantcomponentofhazepollutionwhichisoccurringfrequentlyinWuhan,China.Therefore,itisessentialtoestimatetheiropticalproperties,composition,andmassconcentration.Consideringmosthazepollutionhappensduringthecoldesttime,weretrievedBrCcolumnarcontentduringwinterinWuhanforthefirsttime.OurmethodbasesonthefactthatBrCshowedthestrongspectraldependenceonUV-lightabsorption.Usingthismethod,wefoundthatBrCmakesupthesmallproportionsoftotalaerosolvolume(lessthan10％).Inthewinterof2011,weretrievedthedaily-averagedcolumnar-integratedmassconcentrationofBrConcleardayis4.353mg/m2whilethatofhazedayis12.750mg/m2.Accordingtothesensitivitystudy,wefoundthattheresultshighlyreliedontheassumedaerosolrefractiveindex.Toreducetheuncertaintyofthisapproach,weneedtogainabetterunderstandingofthetemporalvariabilityoftheradiationabsorbingcomponentsoftheseaerosolsinthefuture.

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Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of Wuhan

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Retrieval of Brown Carbon based on the aerosol complex refractive indices in the winter of Wuhan

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